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Prof. Dr. Adrian L. Cavalieri
Prof. Dr. Adrian L. Cavalieri
Research Group Leader
Phone:+49 40 8998 5376Fax:+49 40 8998 1958

Original Publication

1.
S. Schulz, I. Grguraš, C. Behrens, H. Bromberger, J. T. Costello, M. K. Czwalinna, M. Felber, M. C. Hoffmann, M. Ilchen, H. Y. Liu, T. Mazza, M. Meyer, S. Pfeiffer, P. Prędki, S. Schefer, C. Schmidt, U. Wegner, H. Schlarb and A. L. Cavalieri
Femtosecond all-optical synchronization of an X-ray free-electron laser

Extreme Timescales Group

FLASH – the first optically synchronized free-electron laser

Researchers of the MPSD contribute to the improvement of the DESY light source

January 20, 2015

Scientists at the Max Planck Institute for the Structure and Dynamics of Matter (MPSD) and DESY have developed and implemented an optical synchronization system for the soft X-ray free-electron laser FLASH, achieving facility-wide synchronization with femtosecond precision. A femtosecond is a billionth of a microsecond. The performance of the system is expected to ultimately be at least ten times better than what has been achieved anywhere so far using electronic techniques. At this level of control, ultrafast experiments can be performed systematically with the highest temporal resolution, as the team led by Holger Schlarb and Sebastian Schulz from DESY’s machine control and linear accelerator research groups and Adrian Cavalieri from the MPSD reports in the journal Nature Communications.

Free-electron lasers (FELs) generate ultrashort and ultra-intense laser-like light pulses by sending fast electrons from a particle accelerator through a magnetic slalom course. In each bend, the particles emit tiny flashes of light that add up to a strong laser-like pulse. X-ray FELs can be used to reveal the dynamics of the microcosm, such as chemical reactions or properties of biomolecules. For these investigations, however, the timing of the pulses and all the components of the facility must be synchronized with the highest possible precision.

Artistic illustration of the precise clock signal for facility-wide synchronization. A train of near-infrared femtosecond pulses is transmitted on an optical fiber network to the remote locations at the accelerator. To benchmark the performance of the all-optical synchronization system, the relative arrival time between a synchronized optical laser pulse and an X-ray pulse is measured. For comparison, the orange curve is acquired using conventional synchronization, while for the blue curve the all-optical synchronization is active. The narrower the line, the more precise the synchronization.
Artistic illustration of the precise clock signal for facility-wide synchronization. A train of near-infrared femtosecond pulses is transmitted on an optical fiber network to the remote locations at the accelerator. To benchmark the performance of the all-optical synchronization system, the relative arrival time between a synchronized optical laser pulse and an X-ray pulse is measured. For comparison, the orange curve is acquired using conventional synchronization, while for the blue curve the all-optical synchronization is active. The narrower the line, the more precise the synchronization. [less]

In this key demonstration, the optical synchronization system locked all independent accelerator subsystems and external experiment lasers with a precision of 28 femtoseconds – a mere fraction of the X-ray FEL pulse duration of 90 femtoseconds. So far, accelerator facilities and X-ray FELs have primarily been synchronized using electronic radio-frequency clock signals. The best synchronization achieved in this way is limited to about 100 femtoseconds – a restriction that prevents the use of FELs at their full potential for certain applications and inhibits their future development.

The optical synchronization generally improves the characteristics of the X-ray FEL pulses, including arrival time stability, photon energy, intensity, and pulse duration. From the experimentalists’ perspective, however, delivering X-ray pulses with stable properties at exactly the right time is only half of the challenge. The other half rests in the ability to simultaneously deliver an independent optical laser pulse, which is required to initiate ultrafast processes including chemical reactions in molecules and phase transitions in materials. The evolution of these complex dynamics can then be observed using the X-ray FEL pulse. To achieve the maximum time resolution in these studies, ideally, the optical laser pulse should be delivered with a timing precision that is a fraction of the X-ray FEL pulse duration. And the optical synchronization system now demonstrated at FLASH does just that.

Crucially, the team found that the quality of the optical synchronization is limited primarily by the X-ray FEL pulse duration, meaning that the precision should be even better with shorter X-ray pulses. This level of control will not only allow ultrafast experiments with highest temporal resolution, but also open up new possibilities for FEL development. An optical synchronization system based on this prototype will be implemented in the European XFEL, Europe’s future X-ray laser, currently under construction from the research campus Hamburg Bahrenfeld to the neighboring town of Schenefeld.

 
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